Light-Induced Processes in Optically-Tweezed Aerosol Droplets

Light-Induced Processes in Optically-Tweezed Aerosol Droplets

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in Vorbereitung

Aerosols play a critical role in a broad range of scientific disciplines, such as atmospheric chemistry and physics, combustion science, drug delivery and human health. This thesis explores the fundamentals of a new technique for capturing single or multiple particles using light, and for characterising these particles by Raman or fluorescence spectroscopy. The outcome of this research represents a significant development in optical manipulation techniques, specifically in optical tweezing. These findings can be applied to studies of the mass accommodation of gas-phase water molecules adsorbing onto a water surface. Not only is this a fundamental process of interest to physical chemists, but it is important for understanding the role of aerosol particles in the atmosphere, including their ability to become cloud droplets. This new strategy for investigating aerosol dynamics is fundamental in helping us understand the indirect effect of aerosols on the climate.

<p>Introduction</p><p>Aerosol mass transfer</p><p>Experimental techniques </p><p>Optical manipulation in aerosol optical tweezers</p><p>Spectroscopy of optically-tweezed aerosol droplets containing fluorescent chromophores</p><p>Ultra-sensitive absorption spectroscopy of optically-tweezed aerosol droplets</p><p>Kinetics of aerosol mass transfer</p><p>Summary, conclusions and future directions</p>
ISBN 978-3-642-16347-0
Artikelnummer 9783642163470
Medientyp Buch
Auflage 2011
Copyrightjahr 2011
Verlag Springer, Berlin
Umfang XII, 204 Seiten
Abbildungen XII, 204 p.
Sprache Englisch